The striker took his tally to 19 in the Premier League and 22 in all competitions for the season with a match-winning brace either side of half-time at Villa Park.
Dele Alli provided the assist for both goals and was second in the running in the poll with over 19,000 votes from Facebook, Twitter and the Match Centre.
Below: Harry and Dele with Spurs TV at Villa
MAN OF THE MATCH RESULT - VILLA AWAY
Harry Kane - 52.62%
Dele Alli - 18.42%
Kyle Walker - 17.09%
Erik Lamela - 11.87%
Thanks for your votes!
Below - graphic of Harry Kane's second goal